Density profiles of Ar adsorbed in slits of CO2: spontaneous symmetry breaking revisited.

نویسندگان

  • Leszek Szybisz
  • Salvador A Sartarelli
چکیده

A recently reported symmetry breaking of density profiles of fluid argon confined by two parallel solid walls of carbon dioxide is studied. The calculations are performed in the framework of a nonlocal density functional theory. It is shown that the existence of such asymmetrical solutions is restricted to a special choice for the adsorption potential, where the attraction of the solid-fluid interaction is reduced by the introduction of a hard-wall repulsion. The behavior as a function of the slit's width is also discussed. All the results are placed in the context of the current knowledge on this matter.

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عنوان ژورنال:
  • The Journal of chemical physics

دوره 128 12  شماره 

صفحات  -

تاریخ انتشار 2008